Musically, "Gangsta's Paradise" contained an interpolation of Stevie Wonder's 1976 hit "Pastime Paradise" from his critically acclaimed album Songs In The Key Of Life. The hook of "Gangsta's Paradise" was identical to Stevie Wonder's hit except for the word "pastime" being replaced with "gangsta."
L.V. sang the hook and was listed and credited as a featured artist on Coolio's hit. L.V., whose birth name is Larry Sanders was a member of South Central Cartel with Havocc, Prodeje, DJ Kaos and DJ Gripp. In 1995 Coolie told talk show host Howard Stern that he heard L.V. singing the hook and was inspired to write the song. "L.V. was singing the track and I walked in and I was like damn I like that", he explained. Coolio performed "Gangsta's Paradise" live with L.V. at the 38th annual Grammy Awards.